Please use this identifier to cite or link to this item: http://hdl.handle.net/11455/16675
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dc.contributor楊吉斯zh_TW
dc.contributorJyisy Yangen_US
dc.contributor何佳安zh_TW
dc.contributor吳靖宙zh_TW
dc.contributor吳立真zh_TW
dc.contributorJa-an Annie Hoen_US
dc.contributorChing-Chou Wuen_US
dc.contributorLi-Chen Wuen_US
dc.contributor.advisor曾志明zh_TW
dc.contributor.advisorJyh-Myng Zenen_US
dc.contributor.author蘇答zh_TW
dc.contributor.authorPrasad, Sudhakaraen_US
dc.contributor.other中興大學zh_TW
dc.date2009zh_TW
dc.date.accessioned2014-06-06T06:55:55Z-
dc.date.available2014-06-06T06:55:55Z-
dc.identifierU0005-1901200917021800zh_TW
dc.identifier.citationReferences [1] R. W. Murray, Acc. Chem. Res. 13 (1980) 135. [2] R. W. Murray, Chemically Modified Electrodes, Electroanalytical Chemistry, Vol. 13, A. J. Bard, ed., Marcel Dekker Inc., NY, 1984. [3] R. W. Murray, A. G. Ewing, and R. A. Durst, Anal. Chem. 59 (1987) 379A. [4] J. G. Redepenning. Trends Anal. Chem. 6 (1987) 18. [5] N. Oyama, F. C. Anson, Anal. Chem. 52(1980) 1192. [6] R. A. Durst, A. J. Baumner, R. W. Murray, R. P. Buck, C. P. Andrieux , Pure & Appl. Chem. 69 (1997) 1317. [7] J.-M. Zen, A. S. Kumar, D.-M. Tsai, Electroanalysis 15 (2003) 1073 and references there in. [8] J. Wang, Analyst 119 (1994) 763. [9] J. P. Hart, S. A. Wring, Trends Anal. Chem. 16 (1997) 89. [10] K. C. Honeychurch, J. P. Hart, Trends Anal. Chem. 22 (2003) 456. [11] O. D. Renedo, M.A. Alonso-Lomillo, M.J. Arcos Mart´ınez, Talanta 73 (2007) 202. [12] J.-M. Zen, A.S. Kumar, Screen-printed electrochemical sensor, Encyclopedia of Sensors, A.G.Craig, C.D. Elizabeth, V.P. Michael, American Scientific Publisher, California, 2005.zh_TW
dc.identifier.urihttp://hdl.handle.net/11455/16675-
dc.description.abstractScreen printed-carbon electrodes (SPCE) represent a new kind of research tool for electroanalysis due to versatility like fast, simple, disposable and user-friendly nature. The doctoral research emphasized on modification of SPCE by different methods as well as their morphological aspects and applications. Electrochemical activation and oxygen plasma exposition of SPCE revealed the roles of oxygen functionalities and edge-plane sites. Surface bound carbon-oxygen functional groups and generation of edge-plane sites through surface reorientation makes the electrode more electroactive towards NADH, ascorbic acid, dopamine and uric acid. Study of Nafion mixed metal oxide composite-SPCE depicted the structural morphology and catalytic performance towards biologically important thiol (cysteine), disulfide (cystine) and drug analysis of terbutaline. The last phase of doctoral research focused on voltammetric studies and the availability of an on-line single use disposable sensor by shewanella sp. modified SPCE. In brief, the application of electrochemical techniques for developing disposable chemical and bio-sensors is carried out successfully. Most important outcome from the present work is, the activated SPCE shows edge-plane functional group properties, having advantage in simple and fast analysis of various biological /environmental compounds of significance.en_US
dc.description.tableofcontentsCHAPTER 1 1-11 Introduction CHAPTER 2 12-13 Experimental CHAPTER 3 14-26 Mediatorless catalytic oxidation of NADH at a disposable electrochemical sensor CHAPTER 4 27-38 The role of oxygen functionalities and edge plane sites on screen-printed carbon electrodes for simultaneous determination of dopamine, uric acid and ascorbic acid CHAPTER 5 39-59 Direct Electrocatalytic Oxidation of Cysteine and Cystine Based on Nafion/Lead Oxide-Manganese Oxide Combined Catalyst CHAPTER 6 60-71 Sensitive Detection of Terbutaline Using Nafion Pb/MnOx Modified Screen-Printed Carbon Electrode CHAPTER 7 72-83 Direct electron transfer at Shewanella sp. modified screen-printed carbon electrode prepared by a simple drop-coating procedure for sensor application CHAPTER 8 84-89 Conclusions and Further extensionsen_US
dc.language.isoen_USzh_TW
dc.publisher化學系所zh_TW
dc.subjectScreen printed-carbon electrode, Electrochemical / bio sensor, Electroanalysis, Modified electrodesen_US
dc.titleModified Screen-Printed Carbon Electrodes for Electrochemical Sensingen_US
dc.typeThesis and Dissertationzh_TW
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