Please use this identifier to cite or link to this item: http://hdl.handle.net/11455/5906
標題: 高溫好氧薄膜系統對污泥中難分解有機物之處理成效評估
Evaluation of recalcitrants in wasted sludge with a Thermophilic Aerobic Membrane System
作者: 林憶伶
Lin, Yi-Ling
關鍵字: 高溫好氧薄膜系統;the thermophilic aerobic membrane system;鄰苯二甲酸酯類鄰苯二甲酸二乙酯;最大比基質利用率;PCR-DGGE;phthalate esters;diethyl phthalate;maximum specific substrate utilization rate;PCR-DGGE
出版社: 環境工程學系所
引用: 王宇萱(2008)“高溫好氧處理對造紙纖維廢水之可行性初步研究” 碩士論文,國立中興大學環境工程學系,台中。 吳勇興(2004)“自發性高溫好氧處理程序之研究:系統參數測定演算法之開發”博士論文,國立中興大學環境工程學系,台中。 沈育資(2008)“高溫好氧油脂分解菌動力參數研究” 碩士論文,國立中興大學環境工程學系,台中。 林志高(2003)“利用生物與堆肥程序處理都市污水污泥中鄰苯二甲酸酯類化合物及其後續綠農地利用之可行性研究(2/3)”行政院國家科學委員會專題計畫成果報告,國立交通大學環境工程研究所,新竹。 林宜儒(2004)“生物固體物做為受污染土壤生物復育添加劑之可行性探討” 碩士論文,國立中興大學環境工程學系,台中。 林建三(2004)“環境工程概論” 鼎茂圖書出版股份有限公司,台北。 林純志(2006)“單滴溶劑微萃取法結合氣相層析串聯質譜儀檢測水樣中多種鄰苯二甲酸酯類” 碩士論文,私立東吳大學微生物學系,台北。 林慈儀(2008)“高溫好氧系統生物分解動力學及菌相分析之研究” 碩士論文,國立中興大學環境工程學系,台中。 林慧蓉(2009)“評估高溫好氧系統對高濃度有機廢水處理成效及菌相分析研究” 碩士論文,國立中興大學環境工程學系,台中。 邱馨宜(2003)“以微透析裝置連結高效能液相層析儀檢測塑膠容器中飲品之鄰苯二甲酸酯類含量” 碩士論文,國立高雄師範大學化學系,高雄。 施善瑞(2010)“高溫好氧薄膜系統對高濃度有機廢水處理成效之研究” 碩士論文,國立中興大學環境工程學系,台中。 徐振盛、李孟諺(1995)“環境微生物學” 淑馨出版社,台北。 張碧芬,廖健森,柳家瑞,王世冠 (2000)“河川環境鄰苯二甲酸酯類化合物之調查及生物降解之研究”微生物與環境賀爾蒙研討會,pp. 50-59。 張雅雰(2011)“高溫好氧薄膜程序處理生物難分解有機物之研究” 碩士論文,國立中興大學環境工程學系,台中。 張嘉玲(2008)“生物薄膜反應槽薄膜積垢中微生物族群分析研究”,碩士論文,國立交通大學環境工程學系,新竹。 許以樺(2000)“以高溫好氧處理油脂廢水可行性研究” 碩士論文,國立中興大學環境工程學系,台中。 陳國誠(1991)“廢水生物處理學” 國立編譯館,台北。 童永黔,何公亮,曾仁國,劉信堂,吳江饡,李文章 (2002) “污泥最終處置最佳方案評估計劃-污泥堆肥化研究” 工務局衛生下水道工程處研究計畫,台北。 程郁璁(2005)“厭氧生物處理四氯乙烯代謝機制及菌相之探討” 碩士論文,國立中興大學環境工程學系,台中。 黃怡鈞(2008)“鄰苯二甲酸酯類於淡水河紅樹林底泥生物降解之研究” 碩士論文,私立東吳大學微生物學系,台北。 廖健森(2002)“環境荷爾蒙鄰苯二甲酸酯類化合物於台灣水體環境中含量調查與微生物分解之研究” 碩士論文,私立東吳大學微生物學系,台北。 鄭如琇(2006)“以微生物組成探討厭氧發酵系統之產氫效能” 碩士論文,國立中興大學環境工程學系,台中。 鄭曉芬(1999)“以超臨界流體萃取技術萃取都市下水污泥中鄰苯二甲酸-2- 乙基己酯(DEHP)之研究”碩士論文,國立交通大學環境工程研究所,新竹。 顏振義(2002)“高溫好氧消化降解污泥中鄰苯二甲酸酯類之研究” 碩士論文,國立交通大學環境工程學系,新竹。 Abar S., and Satya P.S. (1992) “Environ” Contam Toxicol 48: 115 Ahn, Y., E. J. Park, Y. K. Oh, S. Park, G. Webster, and A. J. Weightman (2005) “Biofilm microbial community of a thermophilic trickling biofilter used for continuous biohydrogen production” FEMS Microbiol. Lett. 249 : 31-38. Amann, R., H. Lemmer, and M. Wagner (1998) “Monitoring the community structure of wastewater treatment plants: a comparison of old and new techniques” FEMS Microbiol. Ecol. 25 : 205-215. Awad, G.A., and Saunders, E.B. (1989) “Adolescent child molesters: Clinical observations”Child Psychiatry and Human Development 19 : 195-206. Baier, U., and Zwiefelhofer, H. D. (1991) “Sludge stabilization, effects of aerobic thermophilic pretreatment” Water Science and Technology 3: 56-61. Banat, F., S. Prechtl, F. Bischof (1999) “Experimental assessment of bio-reduction of di-2-ethylhexyl phthalate (DEHP) under aerobic thermophilic conditions” Chemosphere 39: 2097–2106. Banat, F. A., S. Prechtl, and F. Bischof (2000) “Aerobic thermophilic treatment of sewage sludge contaminated with 4-nonylphenol” Chemosphere 41 : 297-302. Barr, T. A., J. M. Taylor, and S. J. B. Duff (1996) “Effect of HRT, SRT and temperature on the performance of activated sludge reactors treating bleached kraft mill effluent” Wat. Res. 30 : 799–810. BeaT., M. Blanc, P.-F. Lyon, G. Vogt, M. Marchiani, J. L. Fischer and M. Aragno (1996) “ Isolation of Thermus strains from hot composts (60 to 808C) ” Appl. Environ. Microbiol 62: 1723-1727. Beaudet R., C. Gagnon, J. G. Bisaillon and M. Ishaque (1990) “Microbiological aspects of aerobic thermophilic treatment of swine waste” Appl. Environ. Microbiol. 56: 971-976. Bérubé, P. R. and E. R. Hall. (1999) “Treatment of evaporator condensate using a high temperature membrane bioreactor: determination of maximum operating temperature and system costs” In: Proceedings of TAPPI 1999 International Environmental Conference, Toronto, Canada., pp 769–80. Boogerd, F.C., P. Bos, J.G. Kuenen, J.J.Heijnen, R.G.J.M. Van der Lans (1990) “Oxygen and carbon dioxide mass transfer and the aerobic, autotrophic cultivation of moderate and extreme thermophiles: a case study related to the microbial desulfurization of coal” Biotechnol. Bioeng. 35: 1111 – 1119. Brock, T. D., and K. L. Boylen (1973) “Presence of thermophilic bacteria in laundry and domestic hot-water heaters” Appl. Microbiol. 25: 72-76 by variovorax paradoxus T4 and sphingomonas yanoikuyae DOS01 isolated from deep-ocean sediments” Ecotoxicology 15: 549–557. Burt, P., M. H. Littlewood, S. F. Morgan, B. N. Dancer, and J. C. Fry (1990) “Venturi aeration and thermophilic aerobic sewage digestion in small-scale reactors” Appl. Microbiol. Biot. 33 : 721-724. Callia, B., B. Mertoglua, K. Roestb, and B. Inancc (2006) “Comparison of long-term performances and final microbial compositions of anaerobic reactors treating landfill leachate” Bioresource Technol. 97: 641-647. Carter, A.W., and I.H. Suffet (1982) “Binding of DDT to dissolved humic materials” Environ. Sci. Technol. 16: 735–740. Cetin, F. D. and G. Sürücü (1990) “Effects of temperature and pH on the settlability of activated sludge flocs” Wat. Sci. Technol. 22 : 249-254. Chang, In-Soung, Pierre Le Clech, Bruce Jefferson, and Simon Judd (2002) “Membrane Fouling in Membrane Bioreactors for Wastewater Treatment” Journal of Environmental Engineering: 1018–1029. Cheryan, M. (1998) “Ultrafiltration and microfiltration handbook” Technion Pub. Co. Cho, J., G. Amy, J. Pellegrino and Y. Yoon (1998) “Characterization of clean and natural organic matter (NOM) fouled NF and UF membranes, and foulants characterization” Desalination 118:101-108. Chu, A., Mavinic, D. S., Ramey, W. D., and Kelly, H. G. (1994) “Volatile fatty acid production in thermophilic aerobic digestion of sludge” Water Research 28: 1513-1522. Chu, A., Mavinic, D. S., Ramey, W. D., and Kelly, H. G. (1996) “A biochemical model describing volatile fatty acid metabolism in thermophilic aerobic design of wastewater sludge” Water Research 30: 1759-1770. Chu, A., Mavinic, D.S., Kelly, H.G., Guarnaschelli, C., (1997) “The influence of aeration and solids retention time on volatile fatty acid accumulation in thermophilic aerobic digestion of sludge” Environ. Technol. 18 : 731–738. Couillard, D. and S. Zhu (1993) “Thermophilic aerobic process for the treatment of slaughterhouse effluents with protein recovery” Environ. Pollut. 79 : 121-126. Colón I., D. Caro, C.J. Bourdony (2000) “Identification of phthalate esters in the serum of young Puerto Rican girls with premature breast development” Environ Health Perspect 108 : 895-900. Cote, P., M.Masini, and D. Mourato (2004) “Comparison of Membrane Options for Water Reuse and Reclamation” Desalination 167 : 1-11. David L.D. (1990) “Environ” Contam Toxicol de Lucas, A., L. Rodriguez, J. Villasenor, and F. J. Fernandez (2005) “Biodegradation kinetics of stored wastewater substrates by a mixed microbial culture” Biochem. Eng. J. 26 : 191-197 Dias, J. C. T., R. P. Rezende, C. M. Silva, and V. R. Linardi (2005) “Biological treatment of kraft pulp mill foul condensates at high temperatures using a membrane bioreactor” Process Biochem. 40 : 1125-1129. Dorigo, U., L. Volatier, and J. F. Humbert (2005) “Molecular approaches to the assessment of biodiversity in aquatic microbial communities” Wat. Res. 39 : 2207-2218. Dougherty, M. H., and R. R. McNary (1958) “Elevated temperature effect on citrus waste activated sludge” Sewage Indust. Wastes 30: 1263– 1265. Droste, R.L. (1997) “Theory and practice of water and wastewater treatment” John Wiley and Sons Duty, S.M., A.M. Calafat, M.J. Silva, L. Ryan, and R. Hauser (2005) “Phthalate exposure and reproductive hormones in adult men” Hum Reprod. 20: 604–610. Durham, B. and A. Walton (1999) “Membrane Pretreatment of Reverse Osmosis:Long-Term Experience on Difficult Waters” Desalination 122:157-170. Edwars V. H. (1970) “The influence of high substrate concentrations on microbial kinetics ” Biotechnol Bioeng. 12 : 679- 712. Ejlertsson, J.M., S. Alnervik, and B.H. Jonsson (1997) “SvessonInfluence of water solubility, side-chain degradability, and side-chain structure on the degradation of phthalic acid esters under methanogenic conditions” Environ. Sci. Technol. 31: 2761–2764. Epstein, B. A. David, Cannon, W. James, Holt, F. Derek, Levy, V. F. Silvio, Paterson, S. Michael, Thurston, P. William (1992) “Word Processing in Groups, Boston, MA: Jones and Bartlett Publishers”. Fairbanks, R.G. (1989) “A 17,000-year glacio-eustatic sea level record: influence of glacial melting rates on the Younger Dryas event and deep-ocean circulation” Nature 342: 637−642. Fang, H.H.P. and X.L. Shi (2005) “Pore fouling of microfiltration membrane by activated sludge” Journal of Membrane Science 264: 161–166. Fawzi, A., Banat’, Stepban Prechtl, and Franz Bischof (1999) “Experimental assessment of bio-reduction of di-2-thylhexyl phtealate (DEHP) under aerobic thermophilic conditions” Chemical Engineering. Fawzi A., Banat’, Stephan Prechtl , Franz Bischof (1999) “Aerobic thermophilic treatment of sewage sludge contaminated with 4-nonylpheno” Chemosphere 41: 293-302. Ferris, M. J. and D. M. Ward. (1997) “Seasonal distrbutions of dominant 16S rRNA-defined populations in a hot spring microbial mat examined by denaturing gradient gel electrophoresis” Appl. Environ. Microbiol. 63 : 1375-1381. Fujita, Y., M. Fujita, R. Satoh, K. Maruyama, M.M. Parvez, M. Seki, K. Hiratsu, M. Ohme-Takagi, K. Shinozaki, and K. Yamaguchi-Shinozaki (2005) “AREB1 is a transcription activator of novel ABRE-dependent ABA signaling that enhances drought stress tolerance in Arabidopsis” The Plant Cell 17: 3470-3488. Giam, C.S., E. Atlas, J.R. Powers, M .A., and J.E. Leonard (1984) “Phthalate esters ” Anthropogenic Chemicals. Berlin: 67–142. Graczyk, M., and S.T. Kolaczkowski (1980) “Aerobic thermophilic stabilization of hog manure” Proc. Livestock Waste: 342–345. Grunditz, C., and G. Dalhammar (2001) “Development of nitrification inhibition assays using pure cultures of nitrosomonas and nitrobacter” Water Res 35: 433–440. Gu, J. D., and J. H. Yao (2006) “Degradation of dimethyl terephthalate by Pasteurella multocida Sa and Sphingomonas paucimobilis Sy isolated from mangrove sediment” Int Biodeter Biodegr 56: 158–165. Harris, G.W., W.P.L. Carter, A.M. Winer, J.N. Pitts, U. Platt, and D. Perner (1982) “ Observations of nitrous acid in the los angeles atmosphere and implications for the predictions of ozone-precursor relationships” Environ. Sci. Technol. 16: 414-419. Heinonen-Tanski, H., T. Kiuru, J. Ruuskanen, K. Korhonen, J. Koivunen, and A. Ruokoja¨rvi (2005) ”Thermophilic aeration of cattle slurry with whey and/or jam wastes” Bioresource Technol. 96 : 247–252. Houlihan, J., C. Brody, and B. Schwan (2002) “Not Too Pretty: Phthalates, Beauty Products and the FDA” Environmental Working Group, Coming Clean, and Health Care Without Harm. Available Howell, J. A., H. C. Chua, and T. C. Arnot (2004) “ In situ manipulation of critical flux in a submerged membrane bioreactor using variable aeration rates, and effects of membrane history” JMembr Sci. 242: 13–19. Huber, H., M. Thomm, H. Konig, G. Thies, and K. O. Stetter (1982) “Methanococcus thermolithotrophicus, a novel thermophilic lithotrophic methanogen” Arch. Microbiol. 132 : 47-50. In-Soung Chang, Pierre Le Clech, Bruce Jefferson, Simon Judd (2003) “Membrane Fouling in Membrane Bioreactors for Wastewater Treatment” Journal of Environmental Engineering: 128. Jacangelo, J. G., C. Shankararaman and R. R. Trussell (1998) “Membrane treatment” Civil Engineering: 42-45. Jahren, S., J. Rintala and H. Odegaard (2002) “Aerobic moving bed biofilm reactor treating thermomechanical pulping (TMP) whitewater under thermophilic conditions” Water. Res. 36: 1067-1075. Jain, R., A. Pathak, T. R. Sreekrishnan, and M. G. Dastidar (2010) “Autoheated thermophilic aerobic sludge digestion and metal bioleaching in a two-stage reactor system” J. Environ. Sci. 22 : 230–236. Jobbling, S., T. Reynolds, R. Whites, M. G. Parker, and J. P. Sumpter (1995) “A variety of environmentally persistent chemicals, including some phthalate plasticizers, are weakly estrogenic” Environmental Health Perspectives 103 : 582-587. Jones, W. J., J. A. Leigh, F. Mayer, C. R. Woese, and R. S. Wolfe (1983) “Methanococcus jannaschii sp. nov., an extremely thermophilic methanogen from submarine hydrothermal vent” Arch. Microbiol. 136 : 254-261. Judd, S. (2004) “A review offouling of membrane bioreactors in sewage Treatment” Wat. Sci. Technol. 49 : 229-235. Juteau, P., D. Tremblay, C.B. Ould-Moulaye, J.G. Bisaillon, R. Beaudet (2004) “Swine waste treatment by selfheating aerobic thermophilic bioreactors” Water Res. 38: 539–546 Juteau, P. (2006) “Review of the use of aerobic thermophilic bioprocesses for the treatment of swine waste” Livest. Sci. 102 : 187-196. Kelly,H.G., and R. Warren (1995) “What''s in a Name? –Flexibility” Water Environment and Technology. WEF,7: 46–50. Kimura, K., N. Yamato, H.Yamamura, and Y. Watanabe (2005) “Membrane Fouling in Pilot-Scale Membrane Bioreactors (MBR2) Treating Municipal Wastewater” Environ. Sci. Technol. 39 : 6293-6299. Krahe, M., G. Antranikian and H. Markl (1996) “Fermentation of extremophilic microorganisms” FEMS Microbiol. Rev. 18: 271–285. Kumar, A., S. Kumar, and S. Kumar (2005) “Biodegradation kinetics of phenol and catechol using Pseudomonas putida MTCC 1194” Biochem. Eng. J. 22 : 151-159. Kurian, J., S. Esakku, R. Nagendran, and C. Visvanathan (2005) “A decision making tool for dumpsite rehabilitation in developing countries” Tenth Int’l Wasst Management and Landfill Symposium, Environmental Sanitary Engineering Centre Kurian, R., C. Acharya, G. Nakhla, and A. Bassi (2005) “Conventional and thermophilic aerobic treatability of high strength oily pet food wastewater using membrane-coupled bioreactors” Wat. Res. 39 : 4299-4308. Kurian, R., G. Nakhla, and A. Bassi (2006) “Biodegradation kinetics of high strength oily pet food wastewater in a membrane-coupled bioreactor (MBR)” Chemosphere 65 : 1204-1211. LaPara, T. M. and J. E. Alleman (1999) “Thermophilic aerobic waste treatment, review paper” Wat. Res. 33 : 895-908. LaPara, T.M., A. Konopka, , C.H. Nakatsu, J.E. Alleman (2000) “Effects of elevated temperature on bacterial community structure and function in bioreactors treating a synthetic wastewater” Microbiol. Biotechnol. 24: 140– 145. Le-Clech, P., V. Chen, and T. A. G. Fane (2006) “Fouling in Membrane Bioreactors Used in Wastewater Treatment” J. Membrane Sci. 284 : 17-53. Lee, H.B., and T.E. Peart (1995) “Determination of 4-nonylphenol in effluent and sewage sludge from sewage treatment plants” Anal. Chem. 67: 1976–1980. Lerch, R.A., S.R. Bergmann, and B.E. Sobel (1992) “Delineation of myocardial fatty acid metabolism with positron emission tomography” Mount Kisco, NY, USA:129–153 Li, J., J. D. Gu, L. Pan (2005) “Transformation of dimethyl phthalate, dimethyl isophthalate and dimethyl terephthalate by rhodococcus ruber Sa and modeling the processes using the modified Gompertz model” Int Biodeter Biodegr 55: 223–232. Liao, B. Q., D. M. Bagley, H. E. ,Kraemer, G. G. Leppard, and S. N. Liss (2004) “A Review of Biofouling and its Control in Membrane Separation Bioreactors” Wat. Environ. Res. 76 : 425-436. Liu, S., F. Song, N. Zhu, H. Yuan, and J. Cheng (2010) “Chemical and microbial changes during autothermal thermophilic aerobic digestion (ATAD) of sewage sludge” Bioresource Technology 101 : 9438–9444 Mabey, W.R., J.H. Smith, R. Podoll, H.L. Johnson, Mil, W. Chou, J. Gates, Waight Partridge, and D. Vandenberg (1982) “Aquatic fate process data for organic prority pollutants” Envionmental Protection Agency: 183-184 Maidak, B., J. Cole, T. Lilburn, C. J. Parker, P. Saxman, R, Farris, G. Garrity, G. Olsen, T. Schmidt, and J. Tiedje (2001) “The RDPⅡ(Ribosomal Database Project)” Nucleic Acid Res. 29 : 173-174. Mailhot, G., M. Sarakha, B. Lavedrine, J. Caceres, and S. Malato (2002) “ Fe(III)-solar light induced degradation of diethyl phthalate (DEP) in aqueous solutions” Chemosphere 49 : 525-532. Main, K.M., GK. Mortensen, M.M. Kaleva, K.A. Boisen, I.N. Damgaard, M. Chellakooty, I.M. Schmidt, A.M. Suomi, H.E. Virtanen, D.V. Petersen, A.M. Andersson, J. Toppari, and N.E. Skakkebaek (2006) “Human breast milk contamination with phthalates and alterations of endogenous reproductive hormones in infants three months of age” Environmental Health Perspectives 114:270 Marrot, B., A. Barrios-Martinez, P. Moulin, and N. Roche (2004) “Industrial wastewater treatment in a membrane bioreactor: A review” Environmental Progress 23: 59-68. Mavinic, D. S., P. E. V. Mahendraker, A. Sharma and H.G. Kelly (2001) “Effects of microaerophilic conditions on autothermal thermophilic aerobic digestion process” J. Envir. Eng. 5: 311-316. Metcalf and Eddy (1991) “ Wastewater Engineering. Treatment, Disposal, Reuse” 3rd edition, McGraw-Hill Int. Ed. Mikkelsen, H. and K. Keiding (2002) “The shear sensitivity of activated sludge: an evaluation of the possibility for a standardised floc strength test” Wat. Res. 36 : 2931-2940. Mohaibes, M. and H. Heinonen-Tanski (2004) “Aerobic thermophilic treatment of farm slurry and food wastes” Bioresource Technol. 95 : 245-254. Olsen, G. J., D. J. Lane, S. J. Giovannoni, and N. R. Pace (1986) “Microbial ecology and evolution: a ribosomal RNA approach” Annu. Rev. Microbiol. 40 : 337-365. Oles, J., N. Dichtl, and H.H. Niehoff (1997) “Full scale experience of twostage thermophilic/mesophilic sludge digestion” Water Science and Technology 36: 449–456. Oliver, R., E. May, and J. Williams (2007)“Microcosm investigations of phthalate behaviour in sewage treatment biofilms” Sci. Total Environ 372: 605–614. Ponti, M., and M. Abbiati (2004) “Quality assessment of transitional waters using a benthic biotic index: the case study of the Pialassa Baiona (Northern Adriatic Sea) ” Aquatic Conservation: Marine and Freshwater Ecosystems 14: S31-S41. Poulsen, L.K., G. Ballard, and D.A. Stahl (1993) “Use of rRNA fluorescence in situ hybridization for measuring the activity of single cells in young and established biofilms” Appl Environ Microbiol 59: 1354–1360. Qunhui Wang, Kuninobu Masaaki, Kakimoto Kohji, I.-Ogawa Hiroaki, Kato Yasuhiko (1999) “Upgrading of anaerobic digestion of waste activated sludge by ultrasonic pretreatment” Bioresource Technology: 309–313. Ramesh, A., D. J. Lee, and S. G. Hong (2006) “Soluble microbial products (SMP) and soluble extracellular polymeric substances (EPS) from wastewater sludge” Microbiol Biotechnol 73: 219–225. Rittmann, B. E., and P. L. McCarty (2001) Environmental Biotechnology: Principles and Application McGRAW-HILL INTERNATIONAL EDITIONS, Singapore16 : 339. Rosenberger, S., U. Kruger, R. Witzig, W. Manz, U. Szewzyk, M. Kraume (2002) “Performance of a bioreactor with submerged membranes for aerobic treatment of municipal waste water” Water Res 36: 413–420. Rosenberger, S. and M. Kraume (2003) “Parameters influencing filterability of activated sludge in membrane bioreactors” AWWA Membrane Technology Conference. Roslev, P., P.L. Madsen, J.B. Thyme, and K. Henriksen (1998) “Degradation of phthalate and di-(2-ethylhexyl) phthalate by indigenous and inoculated microorganisms in sludgeamended soil” Applied and Environmental Microbiology 64: 4711–4719. Rozich A. F., Clay S. G. and Colvin R. J. (1992) “Thermophilic aerobic treatment of high-strength groundwater: Bench-scale results” 47th Industrial Waste Conference. Rozich, A. F. and R. J. Colvin (1997) “Design and oper-ational considerations for thermophilic aerobic reactors treating high strength wastes and sludges” In Proceedings of the 52nd Industrial Waste Conference. Rozich, A. F. and K. Bordacs (2002) “Use of thermophilic biological aerobic technology for industrial wastewater treatment” Wat. Sci. Tech. 46 : 83-89. Sakol, D. and K. Konieczny (2004) “Application of coagulation and conventional filtration in raw water pretreatment before microfiltration membranes” Desalination 162:61-73. Salles, J. F., F. A. De Souza, and J. D. van Elsas (2002) “Molecular method to assess the diversity of Burkholderia species in environmental samples” Appl. Environ. Microbiol. 68 : 1595-1603. Shugen Liu, Fanyong Song, Nanwen Zhu, Haiping Yuan, Jiehong Cheng (2010) “Chemical and microbial changes during autothermal thermophilic aerobic digestion (ATAD) of sewage sludge” Bioresource Technology101: 9438-9444. Shugen Liu, Nanwen Zhu, Loretta Y. Li (2011) “The one-stage autothermal thermophilic aerobic digestion for sewage sludge treatment: Stabilization process and mechanism” Bioresource Technology104: 266-273. Skjelhaugen, O. J. (1999) “Thermophilic aerobic reactor for processing organic liquid wastes” Wat. Res. 33 : 1593-1602 Staples, C. A., D. R. Peterson, T. F. Parkerton, and W. J. Adams (1997) “The environmental fate of phthalate esters : A literature review” Chemosphere 35 : 667-749 Stenstrom, M. K. and R. G. Gilbert (1981) “Effects of alpha, beta, and theta factor upon the design, specification and operation aeration systems” Wat. Res. 15 : 643-654. Strauch, M. A. (1993) “Regulation of bacillus subtilis gene expression during the transition from exponential growth to stationary phase” Prog Nucleic Acid Res Mol Biol 46: 121–153. Sürücü, M. H., E. S. K. Chian, and R. S. Engelbrecht (1976) “Aerobic thermophilic treatment of high strength wastewaters” J. WPCF 48 : 669-679 Sürücü, G. (1999) “Growth requirements of thermophilic aerobic microorganisms in mixed cultures for the treatment of strong wastes” Wat. Sci. Tech. 40 : 53-60. SuÈ ruÈ cuÈ G. A., Chian E. S. K. and Engelbrecht R. S. (1976) “ Aerobic thermophilic treatment of high strength wastewaters” Wat. Pollut. Control Fed : 669-679. Suvilampi, J. and J. Rintala (2002) “Comparison of activated sludge process at different temperatures: 35℃, 27-55℃, and 55℃” Environ. Technol. 23 : 1127-1134. Suvilampi, J., A. Lehtomäki, and J. Rintala (2003) “Comparison of laboratory-scale thermophilic biofilm and activated sludge processes integrated with a mesophilic activated sludge process” Bioresource Technol. 88 : 207-214. Suvilampi, J., A. Lehtomaki, J. Rintala (2005) “Comparative study of laboratory-scale thermophilic and mesophilic activated sludge processes” Water Resources 39: 741–750. Tchobanoglous, G., F. L. Burton, and D. H. Stensel (2003) Wastewater Engineering Treatment and Reuse, 4th ed. The McGraw-Hill Companies, New York, U.S.A.. Tischer, R. G., L. R. Brown and D. W. Cook (1962) “Decomposition of wastewater by thermophilic microor-ganisms” Wat. Pollut. Control Fed. 34: 1244-1255 Thomas H. S., Judd S., J. Murrer (2000) “Fouling characteristics of membrane filtration in membrane bioreactors” Membrane Technol. 122:10-13. Torsvik, V., J. Goksøyr, and F. L. Daae (1990) “High diversity in DNA of soil bacteria” Appl. Environ. Microbiol. 56 : 782–787. Torsvik, V., L. Øvreas, and T. F. Thingstad (2002) “Prokaryotic diversity - magnitude, dynamics and controlling factors” Science 296 : 1064-1066. Tripathi, C. and D.Allen, (1999) “Comparison of mesophilic and thermophilic aerobic biological treatment in sequencing batch reactors treating bleached kraft pulp mill effluent” Wat. Res. 33 : 836–846. U.S. EPA (1984) “Use and disposal of municipal wastewater sludge” EPA 625/10-84-003. US EPA (1992) “Control of pathogens and vector attraction in sewage treatment” EPA/625/R-92/013 Vega, D., and J. Bastide (2003) “Dimethylphthalate hydrolysis by specific microbial esterase” Chemosphere 51: 663–668. Visvanathan, C., M. K. Choudhary, M. T. Montalbo, and V. Jegatheesan (2007) “Landfill leachate treatment using thermophilic membrane bioreactor” Desalination 204 : 8-16 Vogelaar, J. C. T., A. Klapwijk, J. B. Van Lier, and W. H. Rulkens (2000) “Temperature effects on the oxygen transfer rate between 20 and 55℃” Wat. Res. 34 : 1037-1041. Vogelaar, J., J. van Lier, A. Klapwijk, M. de Vries, and G. Lettinga (2002) “Assessment of effluent turbidity in mesophilic and thermophilic activated sludge reactors-origin of effluent colloidal material” Appl. Microbiol. Biotechnol. 59 : 105-111. Wackett, L. P. and Hershberger, C.D. (2001) “Biocatalysis and biodegradation: microbial transformation of organic compounds” Washington DC: ASM Press. Wang, S. J. and K. C. Loh (1999) “Modeling the role of metabolic intermediates in kinetics of phenol biodegradation” Enzyme Microb. Tech. 25 : 177-184. Wang, J., L. Chen, H. Shi, Qian, and Yi, (2000) “Microbial degradation of phthalic acid esters under anaerobic digestion of sludge” Chemosphere 41 : 1245-1248. Wang ,Y. P., and J. D. Gu (2006) “Degradability of dimethyl terephthalate. Wang, Z.-Y., D. Kenigsbuch, L. Sun, E. Harel, M.S. Ong, and E.M. Tobin (1997)“ A Myb-related transcription factor is involved in the phytochrome regulation of an Arabidopsis Lhcb gene” Plant Cell 9: 491–507. Watanabe, H., T. Kitamura, S. Ochi, and M. Ozaki (1997) “Inactivation of pathogenic bacteria under mesophilic and thermophilic conditions” Water Science and Technology: 3625–3632. Wolf, O.T., B.M. Kudielka, D.H. Hellhammer, J. Hellhammer, and C. Kirschbaum (1999) “Opposing effects of DHEA replacement in elderly subjects on declarative memory and attention after exposure to a laboratory stressor” Psychoneuroendocrinology 23: 617–629. Wynn, B. F., W. V. Linden, and R. C. Backman (1997) “Evaluation of the oxygen transfer characteristics of aeration systems operating in thermophilic temperature ranges”. In Proceedings of the 52nd Industrial Waste Conference. Yamamoto, K. (1994) “Membrane filtration. In rapid filtration, biological filtration and membrane filtration” Gihodo Shuppan. Yamamoto, K., M. Hiasa, T. Mahmood, and T. Matsuo(1989) “Direct solid-liquid separation using hollow fiber membrane in an activated-sludge aeration tank” Water Science and Technology 21: 43–54. Yamagiwa, K., Y., Oohira, A., Ohkawa (1995) “Simultaneous removal of carbonaceous and nitrogenous pollutants by a plunging liquid jet bioreactor with cross-flow filtration operated under intermittent aeration” Bioresource Technol. 53 : 57-62. Yan,C. T. and J. F. Jen (1990) “Analysis of volatile fatty acid in landfill leachates by chromatography”. Yang, W., and N. Ilg J. Cicek (2006) “State-of-the-art of membrane bioreactors: Worldwide research and commercial applications in North America” Journal of Membrane Science 270: 201–211. Yuan, S. Y., C. S. Liu, and B.V. Chang (2002) “Occurrence and microbial degradation of phthalate esters in Taiwan river sediments” Chemosphere 49 : 1295-1299. Yilmaz, T., A. Yuceer, and M. Basibuyuk (2008) “A comparison of the performance of mesophilic and thermophilic anaerobic filters treating papermill wastewater” Bioresource Technol. 99 : 156-163 Zita, A. and A. Hermansson (1997) “Effects of bacterial cell surface structures and hydrophobicity on attachment to activated sludge flocs” Appl. Environ. Microbiol. 63 : 1168-1170.
摘要: 
活性污泥法因應處理各種不同廢水而有不同的處理程序組合及操作條件,但均會產生大量廢棄生物污泥,污泥的後續利用與處置所需要花費的成本頗高,而環境中的難分解污染物質也易累積在污泥之中,因此污泥的減量及其所含之難分解污染物質之降解為本研究目標。鄰苯二甲酸酯類 ( phthalate esters, PAEs ) 化合物常做為塑化劑添加在塑膠製品中,PAEs與高分子塑膠聚合物之間易受時間、溫度等影響,而逐漸釋放到環境水體中,因此本研究選用PAEs之鄰苯二甲酸二乙酯 ( diethyl phthalate, DEP ) 為目標污染物進行生物性降解試驗,並利用高溫好氧薄膜系統 ( thermophilic aerobic membrane system, TAMS ) 消化處理污泥與污泥中之DEP。
高溫好氧薄膜反應槽之有效體積為25 L,溫度控制於55℃,並先以麩胺酸及蔗糖做為進流基質(COD ≒ 10,000 mg/L)進行水相馴養,而後再以同濃度COD之污泥為進流基質。但因系統處理效果不佳,因此系統重新植種高溫菌液且將系統溫度控制為45℃,並將進流基質改為麩胺酸、蔗糖及廢棄污泥。系統定期監測各項水質參數以觀察系統中微生物對污泥及難分解有機物降解之成效。此外,本實驗利用批次試驗求取高溫好氧薄膜系統中微生物於不同COD濃度(麩胺酸、蔗糖及廢棄污泥)之反應動力參數,並進一步探討文獻中微生物生長動力模式之適用性,且以PCR-DGGE觀察系統菌群組成。
本研究試驗的後期系統進流基質改為麩胺酸、蔗糖及廢棄污泥,此階段系統之MLSS去除率為14%、反應槽內tCOD最高去除率為28%、出流水sCOD平均去除率為99%、污泥中DEP去除效率達90%,且出流水中DEP去除效率達95%,此結果顯示高溫好氧薄膜系統對污泥之降解性不佳,但對難分解有機污染物DEP卻有良好的處理成效。本批次試驗結果所得的qmax值為5.18 mg-sub/mg-cell-day,顯示微生物緩慢降解污泥,當以污泥為基質時無法表現高溫好氧系統之高基質利用率之優勢。

The activated sludge system has different combinations and operating conditions to treat different wastewaters. The objective of this research is study the reduction of wasted sludge and the degradation of refractory organic compounds. Phthalate esters (PAEs) are usually added as plasticizer. It is known that PAEs and macromolecule plastic polymers are easy to separate and release to the environment. Thus the presence of refractory organics, such as PAEs, would be common in the treated wastewaters and sludge. Diethyl phthalate (DEP) was used as the target pollutant in this biodegradation test. A thermophilic aerobic membrane system(TAMS) was employed to degrade DEP in wasted sludge.
In this study, the thermophilic aerobic membrane bioreactor, with a volume of 25 L, was maintained at 55℃. Initially, a mixed thermophilic bacterial culture was acclimated with the influent substrate of 10,000 mg-COD/L which was made of glutamic acid and sucrose. Then the same concentration of the wasted sludge was substituted for the influent substrate. Due to the poor treatment results, the system re-seeded with thermophilic microorganisms. The influent substrate was modified containing glutamic acid, sucrose and wasted sludge. The bioreactor was operated at 45℃. In addition, kinetic model was also determined for this thermophilic aerobic membrane system with a series of batch reactors. Furthermore, PCR-DGGE was applied to determine the microbial communities of mixed culture in the bioreactor.
When the influent substrate was made of glutamic acid, sucrose and wasted sludge, the result showed that the removal efficiency of MLSS was only 14%, the highest removal efficiency of tCOD was 28%. The removal efficiencies of sCOD and DEP in the effluent were 99% and 95%, respectively. The removal rate of DEP in the wasted sludge was 90%. Additionally, the maximum specific substrate utilization rate with 5.18 mg-sub/mg-cell-day was found from the batch test. These results have showed that the thermophilic aerobic system has poor degradation rate of sludge but has good treatment efficiency of DEP.
URI: http://hdl.handle.net/11455/5906
其他識別: U0005-1108201220593000
Appears in Collections:環境工程學系所

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